Second-harmonic generation in graded metal–dielectric films of anisotropic particles

نویسندگان

  • J. P. Huang
  • P. M. Hui
  • K. W. Yu
چکیده

We investigate theoretically the effective second-harmonic generation (SHG) susceptibility in graded films of metal–dielectric random composites with anisotropically shaped particles by invoking the local field effects. Using numerical examples, we demonstrate that in the presence of gradation profiles and/or shape effects, graded metal–dielectric films could be used as novel optical materials for producing a broad structure in both the linear and nonlinear (SHG) response and with an enhancement in the nonlinear response.  2005 Elsevier B.V. All rights reserved. PACS: 42.65.-k; 77.22.Ej; 42.79.Ry; 77.84.Lf

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Effective nonlinear optical properties of graded metal–dielectric composite films of anisotropic particles

We study the effective third-order nonlinear susceptibility of a graded metal–dielectric composite film of anisotropic particles with weak nonlinearity by invoking the local field effects within the Maxwell–Garnett theory. We further numerically demonstrate that the film can serve as a novel optical material to produce a broad structure in both the linear and the nonlinear response and an enhan...

متن کامل

Considerably Enhanced Second-Harmonic Generation in Resonant U-Shaped Nano-Structures

In this paper, we perform a detailed study of the spectral response of the gold U-shaped nano-structures for different geometrical parameters and polarizations in order to obtain significant localization factor in the wavelength 1.55 μm. The obtained near-field distribution of electric fields reveals that resonances in these nano-structures correspond to the even and odd plasmonic modes dependi...

متن کامل

Second-harmonic generation in graded metallic films.

We study the effective second-harmonic generation (SHG) susceptibility in graded metallic films by invoking the local field effects exactly and further numerically demonstrate that graded metallic films can serve as a novel optical material for producing a broad structure in both the linear and the SHG response and an enhancement in the SHG signal.

متن کامل

Optical second harmonic generation studies of ultrathin high-k dielectric stacks

We report an investigation of charge transfer in high-k dielectric stacks on Si by second harmonic generation sSHGd. Ultrathin s2–6 nmd films of HfO2, ZrO2, and Al2O3 grown on Si surfaces by atomic layer deposition were investigated and compared to conventional SiO2-based gate dielectrics. From the SHG rotational anisotropy sSHG-RAd of Si-shigh-kd and Si–SiO2 systems, optical roughness of the f...

متن کامل

Dielectric response of graded spherical particles of anisotropic materials

Anisotropic dielectric response occurs naturally due to the presence of gradation, like in functionally graded materials or graded biological cells. However, these materials with locally anisotropic dielectric responses can have macroscopically isotropic responses. In treating graded particles of anisotropic materials, traditional isotropic gradation methods need to be modified. In this work, w...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:

دوره   شماره 

صفحات  -

تاریخ انتشار 2005